Preliminary comparison of trace metals in coastal aerosols between Qingdao and Liverpool

Changling Liu; Jing Zhang; Roy Chester

doi:10.1007/s00343-008-0203-4

Your Location：

Home >

Browse articles >

Preliminary comparison of trace metals in coastal aerosols between Qingdao and Liverpool

OriginalPaper | Updated：2023-05-16

- Preliminary comparison of trace metals in coastal aerosols between Qingdao and Liverpool
- Preliminary comparison of trace metals in coastal aerosols between Qingdao and Liverpool
- 海洋湖沼学报（英文） 2008年26卷第2期页码：203-214
- Affiliations：
  
  1. Qingdao Institute of Marine Geology
  2. State Key Laboratory of Estuarine and Coastal Research East China Normal University
  3. Oceanography Laboratories Department of Earth Science the University of Liverpool
- Author bio：
- Funds：
  
  Funded by the Ministry of Science and Technology of China (No. G1999043705 and 2001CB-409703) and the Natural Sciences Foundation of Shandong Province (No. 2000E02)
- DOI：10.1007/s00343-008-0203-4
  中图分类号：
- 网络首发：2008-05-28，
  
  纸质出版：2008
- Accepted：
Scan QR Code
Preliminary comparison of trace metals in coastal aerosols between Qingdao and Liverpool[J]. 海洋湖沼学报（英文）, 2008,26(2):203-214.

Liu, C., Zhang, J. & Chester, R. Preliminary comparison of trace metals in coastal aerosols between Qingdao and Liverpool., Chin. J. Ocean. Limnol. 26, 203–214 (2008). https://doi.org/10.1007/s00343-008-0203-4
Preliminary comparison of trace metals in coastal aerosols between Qingdao and Liverpool[J]. 海洋湖沼学报（英文）, 2008,26(2):203-214. DOI： 10.1007/s00343-008-0203-4.

Liu, C., Zhang, J. & Chester, R. Preliminary comparison of trace metals in coastal aerosols between Qingdao and Liverpool., Chin. J. Ocean. Limnol. 26, 203–214 (2008). https://doi.org/10.1007/s00343-008-0203-4 DOI：

摘要

Abstract

Aerosol samples were collected at two coastal suburban stations

Qingdao (China) in 1995–1996 and Liverpool (U.K.) in 1995

respectively. The samples were analyzed to determine the concentrations of trace metals (Cr

and Cd) as well as Al

Fe and Mn. Data were examined to understand the difference of trace metals in aerosols between coastal zones downwind the developing area (near the Yellow Sea) and developed region (near the Irish Sea). The results show that most elements at Qingdao have levels 4–5 times higher than those at Liverpool

particularly for the crust-dominated elements (e.g. Al

Fe and Mn). Moreover

the aerosol composition at Qingdao is higher in spring than in summer

underlying the influence of westerlies and local emissions in combination

whereas seasonal change of aerosol composition is not significant at Liverpool. The enrichment factors for the crustal source elements (EF crust) at Liverpool are much higher than those at Qingdao. The contributions from the pollutant source (R p) for some trace metals like Cu

Zn and Cd are >90% at Qingdao and Liverpool

suggesting overwhelming anthropogenic contributions to these metals. The contributions from crustal source (R c) for trace metals tend to increase with higher aerosol levels and Al concentration at Qingdao

indicating a good correlation between the crust-dominated component and the air mass. At Liverpool

the R c values for trace metals are positively correlated with Al concentrations instead of with aerosol mass

suggesting that Al in aerosols represents the crustal component even though the aerosols come from different sources.

关键词

Keywords

references

Brewer, P., 1975. Minor Elements in Seawater. Chemical Oceanography, 2nd ed., Vol. 1, Riley, J. P. and G. Skirrow, Eds, Academic, NY, p.415–496.

Chen, L. L., G. R. Carmichael, M. S. Hong et al., 1997. Influence of continental outflow events on the aerosol composition at Cheju Island, South Korea. Journal of Geophysical Research 102: 28 551–28 574.

Chen, L. Q., Z. H. Wang, X. L. Yang et al., 1999. Characteristics of metals in atmosphere over the western Taiwan Strait: I Concentration and distribution. Acta Oceanologica Sinica 18(3): 412–422.

Chester, R., G. F. Bradshaw, 1991. Source control on the distribution of particulate trace metals in North Sea atmosphere. Marine Pollution Bulletin 22: 30–36.

Chester, R., M. Nimmo, M. Alarcon et al., 1993. Defining the chemical character of aerosols from the atmosphere of the Mediterranean Sea and surrounding regions. Oceanology Acta 16: 231–246.

Chester, R., M. Nimmo, G. R. Fones et al., 2000. Trace metals chemistry of particulate aerosols from the UK mainland coastal rim of the NE Irish Sea. Atmospheric Environment 34: 949–958.

Chester, R., E. J. Sharples and K. J. T. Murphy, 1984. The distribution of particulate Mo in the Atlantic aerosol. Oceanology Acta 7: 441–450.

Chung, Y. S., 1992. On the observations of Yellow Sand (dust storms) in Korea. Atmospheric Environment, 26A: 2 743–2 749.

Eyckmans, K., J. Zhang, J. D. Hoog et al, 2001. Leaching of nutrients and trace metals from aerosol samples, a comparison between a re-circulation and an ultrasound system. International Journal of Environmental Analytical Chemistry 80(3): 227–243.

Gao, Y., R. Arimoto, R. A. Duce et al., 1992. Input of atmospheric trace elements and mineral matter to the Yellow Sea during the spring of a low-dust year. Journal of Geophysical Research 97: 3 767–3 777.

Gao, Y., R. Arimoto, R. A. Duce et al., 1997. Temporal and spatial distributions of dust and its deposition to the China Sea. Tellus 49B:172–189.

Guieu, C., R. Chester, M. J. Nimmo et al., 1997. Atmospheric input of dissolved and particulate metals to the northwestern Mediterranean. Deep-Sea Research 44(2): 665–674.

Hong, G. H., S. H. Kim, D. B. Yang et al., 1998. Atmospheric input of trace metals over the Yellow Sea: Shipboard results, April 1995. In: Heath of the Yellow Sea, Hong, G. H., et al., eds., The Earth Love Publication Association, Seoul, p. 251–283.

Liu, C. L., 1997. Transport of Particulate Heavy Metals to the Ocean via River and Atmosphere. MSc. thesis, Dept. of Marine Chemistry, Ocean Univ. of Qingdao, Qingdao, 105pp.

Liu, C. L., J. Zhang and Z. B. Shen, 2002. Spatial and temporal variability of trace metals in aerosol from the desert region of China and the Yellow Sea. Journal of Geophysical Research 107(D14)(ACH17), 1–17.

Tanner, P. A. and A. Y. S. Wong, 2000. Soluble trace metals and major ionic species in the bulk deposition and atmosphere of Hong Kong. Water, Air and Soil Pollution 122: 261–279.

Taylor, S. R. and S. M. McLennan, 1995. The geochemical evolution of the continental crust, Reviews of Geophysics 33: 241–265.

Zhang, J., S. Z. Chen, and Z. G. Yu et al., 1999. Factors influencing changes in rainwater composition from urban versus remote regions of the Yellow Sea. Journal of Geophysical Research 104: 1 631–1 644.

Zhang, J. and R. Chester, 2002. Difference of rainwater compositions at Liverpool and Qingdao: A comparison study between the Yellow Sea and the Irish Sea. In: Impact of Interface Exchange on the Biogeochemical Processes of the Yellow Sea, Hong, G. H. et al., eds., Bumshin Press, Seoul, p3–31.

Zhang J., Y. Wu, C. L. Liu et al., 2001. Aerosol characters from the desert region of Northwest China and the Yellow Sea in spring and summer: Observations at Minqin, Qingdao, and Qianliyan in 1995–1996, Atmospheric Environment 35: 5 007–5 018.

Zhang J., Y. Wu, C. L. Liu et al., 2002. Major components of Aerosols in North China: Desert region and the Yellow Sea in the spring and summer of 1995 and 1996. Journal of Atmospheric Sciences 59: 1 515–1 532.

浏览量

Downloads

CSCD

文章被引用时，请邮件提醒。

Submit

工具集

关联资源

Chemical characteristics of aerosols in the Kuroshio area

Effects of Fe and Mn on the growth of a red tide dinoflagellateScrippsiella trochoidea (Stein) Loeblch III

Measurement of labile Cu, Pb and their complexation capacity in Yueqing Bay in Zhejiang Province, China

Molecular phylogenetic analysis of attached Ulvaceae species and free-floating Enteromorpha from Qingdao coasts in 2007

水下超声速气流流场非定常特性研究