Bifunctional nanozyme activities of layered double hydroxide derived Co-Al-Ce mixed metal oxides for antibacterial application

Chao CHEN; Yi WANG; Dun ZHANG

doi:10.1007/s00343-020-0041-6

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Bifunctional nanozyme activities of layered double hydroxide derived Co-Al-Ce mixed metal oxides for antibacterial application

Chemistry | Updated：2023-04-27

- Bifunctional nanozyme activities of layered double hydroxide derived Co-Al-Ce mixed metal oxides for antibacterial application
- Bifunctional nanozyme activities of layered double hydroxide derived Co-Al-Ce mixed metal oxides for antibacterial application
- 海洋湖沼学报（英文） 2020年38卷第4期页码：1233-1245
- Affiliations：
  
  1.CAS Key Laboratory of Marine Environmental Corrosion and Bio-fouling, Institute of Oceanology, Chinese Academy of Sciences, Qingdao 266071, China
  2.University of Chinese Academy of Sciences, Beijing 100049, China
  3.Open Studio for Marine Corrosion and Protection, Qingdao National Laboratory for Marine Science and Technology, Qingdao 266237, China
  4.Center for Ocean Mega-Science, Chinese Academy of Sciences, Qingdao 266071, China
- Author bio：
  
  WANG Yi, wangyi@qdio.ac.cn
  ZHANG Dun, zhangdun@qdio.ac.cn
- Funds：
  
  the Strategic Priority Research Program of Chinese Academy of Sciences(XDA23050104);the National Natural Science Foundation of China(41776090);the National Natural Science Foundation of China(41976032);the Key Research and Development Program of Shandong Province(2018GHY115038);the AoShan Talent Program Supported by Qingdao National Laboratory for Marine Science and Technology;© Chinese Society for Oceanology and Limnology, Science Press and Springer-Verlag GmbH Germany, part of Springer Nature 2020
- DOI：10.1007/s00343-020-0041-6
  中图分类号：
- 收稿：2020-01-21，
  
  录用：2020-3-12，
  
  网络首发：2020-03-21，
  
  纸质出版：2020-07
- Accepted：
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Bifunctional nanozyme activities of layered double hydroxide derived Co-Al-Ce mixed metal oxides for antibacterial application[J]. 海洋湖沼学报（英文）, 2020,38(4):1233-1245.

Chao CHEN, Yi WANG, Dun ZHANG. Bifunctional nanozyme activities of layered double hydroxide derived Co-Al-Ce mixed metal oxides for antibacterial application[J]. Journal of Oceanology and Limnology, 2020, 38(4): 1233-1245.
Bifunctional nanozyme activities of layered double hydroxide derived Co-Al-Ce mixed metal oxides for antibacterial application[J]. 海洋湖沼学报（英文）, 2020,38(4):1233-1245. DOI： 10.1007/s00343-020-0041-6.

Chao CHEN, Yi WANG, Dun ZHANG. Bifunctional nanozyme activities of layered double hydroxide derived Co-Al-Ce mixed metal oxides for antibacterial application[J]. Journal of Oceanology and Limnology, 2020, 38(4): 1233-1245. DOI： 10.1007/s00343-020-0041-6.

摘要

Abstract

Marine biofouling is an expensive problem that needs evolved chemical or physical antifouling strategies. However

most of the current antifouling materials that would damage the environment through metal leaching and bacteria resistance are being halted. Nanozyme is one kind of environmental antifouling materials through generating reactive oxygen species (ROS). We prepared various contents of CeO

that could uniform disperse compounding with Co

and CoAl

to form a stable Co-Al-Ce mixed metal oxide (MMO) by a layered double hydroxide derived method. We find that coupling with CeO

can improve the peroxidase (POx) activity. When the molar ratio of Ce is 2.5% and the calcination temperature is 200¦

the POx activity of Co-Al-Ce MMO is the best caused by the good dispersion of catalytically active components and the high specific area (150.10±4.95 m

/g). This novel Co-Al-Ce MMO also exhibits an antibacterial mode of action Gram-negative bacteria in near-neutral pH solution through generating ROS (mainly ·O

) in the presence of H

. Ce containing MMO can be utilized as potential green marine antifouling material.

关键词

Keywords

references

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